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    北理工楊國昱教授團隊在化學類頂級國際期刊《Accounts of Chemical Research》上發表封面文章

    供稿: 化學與化工學院 編輯: 李亞鑫
    (2019-01-17) 閱讀次數:
    【字號  大

     

      金屬氧合團簇因其具有奇特的物理化學性質,已經成為構造新型分子基功能材料的重要無機構筑單元。其中,以具有磁學及光學等優異性能的稀土氧合團簇為構筑單元的研究引起了化學家與材料學家的廣泛關注和興趣。

      北京理工大學化學與化工學院/原子分子簇科學教育部重點實驗室楊國昱教授研究團隊長期致力于氧合團簇的設計合成與組裝策略等方面的研究。在國家杰出青年科學基金、國家基金委重大研究計劃重點項目、科技部973計劃課題及北京理工大學“簇科學”創新團隊項目的資助下,該團隊在稀土氧合團簇有機骨架領域取得了創新性研究成果。近期,該團隊應邀在具有重要國際影響的化學類頂級國際期刊——美國化學會《化學研究評述》(Accounts of Chemical Research)雜志上發表了題為“簇有機骨架中的誘導聚集成簇和協同配位策略” (Induced Aggregation and Synergistic Coordination Strategy in Cluster Organic Architectures)的綜述文章(Acc. Chem. Res., 2018, 51, 2888-2896, doi: 10.1021/acs.accounts.8b00346)并被選為封面(Cover)文章。這是該團隊多年來在稀土氧合團簇化學領域研究成果與研究經驗的總結,也是我校化學學科在該雜志上發表的第一篇綜述文章。綜述中的部分研究成果是該團隊獲得2016年國家自然科學獎二等獎《氧基簇合物的設計合成與組裝策略》的重要組成部分。

      該綜述總結了團隊多年來在稀土氧合團簇有機骨架領域取得的主要進展,闡述了誘導聚集成簇與協同配位策略的產生和發展。根據“軟硬酸堿理論”,稀土離子易與氧原子配位,而過渡金屬離子更傾向于與氮原子配位。基于此,該團隊選擇了同時具有氮和氧原子的線性有機配體,其中作為電子給體的氧原子可誘導稀土離子聚集成簇,而氮原子給體可誘導過渡金屬聚集成簇,進而成功構建了一系列稀土氧合團簇有機骨架。研究表明:第二配體的引入對第一配體的配位模式及稀土氧合團簇有機骨架類型產生了重要的影響。同時,根據有機配體的不同類型,詳細介紹了第二配體與第一配體間的三種協同作用:(1) 有機配體與有機配體間的協同作用;(2) 有機配體與無機配體間的協同作用;(3) 上述兩種協同作用同時存在。綜述的最后部分對誘導聚集成簇和協同配位策略的未來發展進行了展望,指出該策略具有較好的普適性,已在過渡金屬氧合團簇、稀土-主族氧合團簇有機骨架及晶態鈦氧簇基骨架中得到相應體現。

      上述研究成果不僅提升了北京理工大學在原子簇化學研究領域的國際學術影響力,而且為原子分子簇科學教育部重點實驗室的進一步發展奠定了堅實基礎。

      到目前為止,該團隊已經在Acc. Chem. Res.、Chem. Rev.、Chem. Soc. Rev.、J. Am. Chem. Soc.、Angew. Chem. Int. Ed.、Chem. Commun.、Chem. Eur. J.、Inorg. Chem.、Dalton Trans.、Cryst. Growth Des.及CrystEngComm等有重要影響的國內外雜志上發表氧合團簇化學方面的研究論文300余篇。


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